Still unable to pin-point the exact date. But found a few more information:
1. The Caritas website mentioned the Caine Road Centre was inaugurated in 1963. Uncertain if it was meant for the older building shown or something else;
2. There is a foundation stone, a bit blurred in Street View but still visible, showing it was laid on 19th March 1964;
The Names of Buildings gives 1968 as the completion date for Caritas House, which seems a bit late but not impossible for a 1964 foundation stone.
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